欧美地下水有机污染调查评价进展   总被引：11，自引：0，他引：11  

刘菲  王苏明  陈鸿汉 《地质通报》2010,29(6):907-917

1999年中国地质调查局启动了第一个地下水有机污染调查项目,当时检测指标只有20个(包括11个挥发性有机污染物、8种有机氯农药和1种多环芳烃)。"十一五"的地下水有机污染调查必测项目包含了38项(挥发性指标28项、有机氯农药9项和1种多环芳烃),取得了地下水有机污染的基本资料。但从对国外文献的调研来看,地下水中有机污染的种类远远超过38种。为了更全面地掌握中国地下水的质量,有必要对不同地区或不同类型的地下水中典型的有机污染物的种类进行研究,为后续地下水有机污染调查的增项做准备。通过检索美国环保局(USEPA)、美国地质调查局(USGS)和欧盟(EU)近年来的地下水质量年度报告和相关文献,调研了地下水中典型有机污染物的类型,选出最常检出的有机污染物,形成最常检出的有机污染物的检出率排序表,列出了检出率高的前50个污染物的名单。  相似文献   

Electro‐Oxidation of the Pharmaceutical Furosemide: Kinetics,Mechanism, and By‐Products          下载免费PDF全文

Hugo Olvera‐Vargas  Nihal Oturan  Didier Buisson  Eric D. van Hullebusch  Mehmet A. Oturan 《洁净——土壤、空气、水》2015,43(11):1455-1463

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随机波浪下斯托克司漂移速度是否引起水面漂移物离散的研究     

黄国兴  LAW Wing-Keung Adrian 《海洋学报(英文版)》2018,37(7):55-61

漂浮于自由水面的污染物的的迁移、扩散会受到天然随机海浪的影响。之前的研究（以Herterich和Hasselmann（1982）为代表）普遍认为，随机波浪作用下的斯托克司漂移速度会引起水面污染物的离散，这个离散甚至有可能跟风和海流引起的离散同一量级。本研究就随机波浪作用下的斯托克司漂移速度是否会引起水面漂移物的离散进行理论和试验探讨。从理论推导可知，随机波浪下的质量输移速度是个定常分量，因此它不会随时间变化而引起水面漂移物的离散。随后我们在实验室水槽中进行了漂移物在随机波浪（P-M谱）作用下的漂移过程的测量。试验结果也印证了随机波浪作用下的斯托克司漂移速度不会引起水面漂移物离散的结论。  相似文献   

Chemostatic behaviour of major ions and contaminants in a semiarid spring and stream system near Los Alamos,NM, USA          下载免费PDF全文

Jace M. Koger  Brent D. Newman  Timothy J. Goering 《水文研究》2018,32(11):1709-1716

Recent studies have focused on the relationship between solute concentrations and discharge in streams, demonstrating that concentrations can vary little relative to changes in discharge (chemostatic behaviour). Chemostatic behaviour is dependent on catchment characteristics (e.g., lithology, geomorphology, and vegetation) and chemical characteristics of the solute (e.g., availability, reactivity, and mobility). An investigation of 3 springs and a stream near Los Alamos, NM, reveals that springs can behave in a chemostatic fashion as stream systems tend to do. Another unique finding of this study is that the anthropogenic contaminants barium and the high explosive RDX (hexahydro‐1,3,5‐trinitro‐1,3,5‐triazine) can also behave chemostatically. The chemostatic behaviour of a contaminant has important implications for the residence time of contaminants in a system as well as having a major control on contaminant flux and mass transport. Redox (reduction–oxidation) and biogeochemically sensitive analytes (e.g., Fe, SO₄, and NO₃) display a combination of chemostatic and chemodynamic behaviour, showing the influence of temporally variable conditions on stream and spring chemistries.  相似文献   

The Forest in the Future: A Response to Seeing the Forest for the Trees     

Jessica D. Ulrich-Schad  Jennifer E. Givens 《社会与自然资源》2020,33(9):1154-1161

Abstract

In this commentary, we highlight some of the strengths of the bibliometric analysis conducted by Qin et al. that examines the relationships between environmental and natural resource sociologies through citation networks, coauthorship, and keyword usage. We also suggest some ways that the analysis could be expanded or built upon, and ideas for further distinct, but related, inquiry. We also reflect on our own identification, training, and mentoring within the two subfields and draw upon responses from a small purposefully selected sample of other early/mid-career environmental and natural resource sociologists to start a conversation about what the relationship between the two fields might look like in the future.  相似文献   

Characterization of Organic Contaminants in New York/New Jersey Harbor Sediments Using FTIR‐ATR and Synchrotron FTIR     

Zhiguang Song  Keith W. Jones  Nebojsa Marinkovic  Xian Ming Xiao  Huan Feng  Elli Tchouparova 《洁净——土壤、空气、水》2011,39(12):1041-1049

Dredging and remediation of contaminated Harbor sediments requires characterization of organic pollutants. In this paper, we apply a combination of Fourier transform IR attenuated total reflectance (FTIR‐ATR) and synchrotron FTIR techniques to the investigation of sediments and related materials from New York/New Jersey Harbor and other locations. The FTIR techniques give information on the functional groups of the compounds found in the sediments and make possible measurements with a spatial resolution of about 0.015 mm. Comparisons of natural organic materials namely, river and groundwater humic substances, recent marine and lacustrine sediments, and ancient sedimentary kerogen show that contaminated NY/NJ Harbor sediments display a strong and distinct absorption in their IR spectra at 2850–2950 cm^?1 identified as a C? H stretching band, indicative of the presence of anthropogenic hydrocarbons. We suggest that the presence of this band could be used for rapid screening for the presence of contaminant organic compounds in sediments encountered in dredging operations and/or as an indicator for the efficacy of sediment decontamination technologies used for treatment of dredged material.  相似文献   

世界主要国家碳排放强度历史变化趋势及相关关系研究   总被引：4，自引：1，他引：3  

张志强  曾静静  曲建升 《地球科学进展》2011,26(8):859-869

减少人类活动的温室气体特别是CO2排放量是国际社会已普遍达成共识的应对气候变暖的根本性途径。研究各国经济活动的碳排放强度的变化历史,可以为预测各国未来的碳排放强度趋势、制定未来的碳排放强度降低目标提供科学依据。利用美国橡树岭国家实验室CO2信息分析中心（CDIAC）的CO2排放数据、《世界人口、国内生产总值和人均国内生...  相似文献   

Emerging organic contaminants (EOCs) in freshwaters in Dunedin,New Zealand     

Melody J. Bernot  Randall J. Bernot  Christoph D. Matthaei 《新西兰海洋与淡水研究杂志》2019,53(1):3-14

Emerging organic contaminants (EOCs) in New Zealand freshwaters are not well documented for regulatory assessments. We collected water and sediment samples for measurement of 26 EOC compound concentrations at four waterways within the city of Dunedin (Otago province). Compounds measured ranged from stimulants and depressants to pain-killers and insect repellants. Sampling was conducted before and after the student ‘Orientation Week’ at the University of Otago. Most compounds were below detection limits in all samples. However, caffeine, carbamazepine, cotinine and DEET were all measured at concentrations above detection limits. In general, concentrations of EOC compounds were ～20% higher following the influx of students to the University though student effects varied by site and additional sampling is needed to better assess temporal variation in concentrations. These data indicate that some EOCs are present in New Zealand freshwater ecosystems.  相似文献   

Environmental recovery in Sydney Harbour,Nova Scotia: Evidence of natural and anthropogenic sediment capping     

Tony R. Walker  Devin MacAskill  Peter Weaver 《Marine pollution bulletin》2013

Contaminants were assessed in Sydney Harbour during baseline and three years of remediation of a former coking and steel facility. Concentrations of PAHs; PCBs; and lead measured in surface sediments indicate overall spatial distribution patterns of historical contaminants remains unchanged, although at much lower concentrations than previously reported due to natural sediment recovery. Recovery rates were in broad agreement with predicted concentrations; or in some cases lower, despite remediation at the Sydney Tar Ponds (STP) site. Contaminants showed little temporal variability, except for detection of significant increases in PAH concentrations during onset of remediation compared to baseline which represented a short term interruption in the overall long term natural recovery of sediments in Sydney Harbour. Recovery (via “capping”) was enhanced following recent harbour dredging activities where less contaminated outer harbour sediments were discharged into a confined disposal facility (CDF) required for a new container in the inner harbour.  相似文献   

还原态蒙脱石有氧条件产生羟自由基降解有机污染物     

袁松虎  姚炜钰  张鹏  刘细祥 《矿物岩石地球化学通报》2019,(3):485-489,439

近期见有含二价铁矿物可活化分子氧产生羟自由基而氧化污染物的报道。本文选用土壤/沉积物中的常见组分蒙脱石(含铁约2%),研究了还原态蒙脱石在不同条件下活化分子氧降解苯酚的效果。结果表明,20g/L还原态蒙脱石(还原程度为30%)在pH=6和有氧条件下,可通过产生羟自由基使11μM苯酚的降解率在6h内持续增加至59.1%。苯酚降解率对应的最佳pH为5,当pH>6时降解率则随着p H的升高而急剧降低;苯酚降解效果还随还原态蒙脱石剂量(0~40g/L)增加而提高;苯酚初始浓度为11μM降解率最高,增加或者降低初始浓度均使降解率降低。还原态蒙脱石铁含量低,活化分子氧时其八面体边缘配位和结构内部二价铁共同起作用,而受八面体层Al、Mg等惰性组分阻碍,其结构二价铁难以向边缘位置传递电子,这与前期报道的还原态绿脱石(含铁约20%)不同。  相似文献